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• W4280590807 endingPage "231614" @default.
• W4280590807 startingPage "231614" @default.
• W4280590807 abstract "All-solid-state thin-film Li-ion batteries (ASSTFBs) have been regarded as a promising power source for microsystems. The main bottleneck of ASSTFBs is that its capacity degrades significantly with decreasing working temperatures, which has been ascribed to the huge mass-transfer overpotential across the solid-state electrolyte because of its low ion conductivity. In this work, a fully coupled electrochemical-mechanical-thermal model is established to investigate the behaviors of ASSTFBs with a typical LiCoO2/LiPON/Li ASSTFB configuration, especially at low temperatures. Numerical simulation is also performed based on this fully coupled model. The simulation results agree well with the experimental data in a wide temperature range (243 K–353 K) and current rate (30 μA cm−2 to 300 μA cm−2), verifying the effectiveness and accuracy of this fully coupled model. Moreover, based on this model, it is found that both mass-transfer overpotential across the electrolyte and charge-transfer overpotential at the cathode/electrolyte interface are the key factors determining the ASSTFB performance at room temperatures; for comparison, the charge-transfer overpotential at the cathode/electrolyte interface plays the dominant role at low temperatures. This work provides a deep insight into the ASSTFB behaviors as well as its performance optimization strategy, particularly at low temperatures." @default.
• W4280590807 created "2022-05-22" @default.
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• W4280590807 date "2022-08-01" @default.
• W4280590807 modified "2023-10-14" @default.
• W4280590807 title "A fully coupled electrochemical-mechanical-thermal model of all-solid-state thin-film Li-ion batteries" @default.
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• W4280590807 doi "https://doi.org/10.1016/j.jpowsour.2022.231614" @default.
• W4280590807 hasPublicationYear "2022" @default.
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