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- W4280593107 abstract "To significantly abate the carbon footprint in the conventional Haber-Bosch process, a novel approach based on wet air co-electrolysis in solid oxide electrolysis cell (SOEC) was proposed and evaluated in this study for sustainable single-step production of ammonia feedstock (i.e., H2/N2 mixture). An electrolyte-supported SOEC composed of LSCM-GDC cathode, SSZ electrolyte and LSCF-GDC anode was prepared and tested under various operation conditions. The current-voltage responses measured for wet air co-electrolysis were featured with three different regions which could be attributed to competitive and combinative effects of oxygen splitting reaction and water splitting reaction under wet air co-electrolysis operation. Gas chromatography (GC) analysis of the exit gas from the cathode chamber proved that high purity H2/N2 mixture had been produced successfully through the novel wet air co-electrolysis process. However, the obtained H2:N2 ratios were still much lower than the desired 3:1 ratio in the ammonia feedstock for the Haber-Bosch process. Further explorations will be made to increase the H2:N2 ratio in the produced gas mixture." @default.
- W4280593107 created "2022-05-22" @default.
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- W4280593107 date "2022-05-01" @default.
- W4280593107 modified "2023-09-26" @default.
- W4280593107 title "Wet-air co-electrolysis in high-temperature solid oxide electrolysis cell for production of ammonia feedstock" @default.
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- W4280593107 doi "https://doi.org/10.1016/j.ijhydene.2022.04.017" @default.
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