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• W4280636120 abstract "Efficient transformation of Fe(III) to Fe(II) enhances the efficiency of persulfate-based Fenton-like process (e.g., Fe(II)-PS system). Here, we developed a novel heterogeneous Fenton-like system driven by visible light (organic-Fe(III)-PS-TiO2-Vis) for effective reduction of Fe(III), activation of PS and degradation of organic pollutants without the need for external reducing agents or modifications in TiO2. The visible light-induced ligand-to-metal (organic-to-TiO2) charge transfer (LMCT) remarkably boosting Fe(III) reduction to increase reactive oxygen species (ROS) via PS activation, and further enhanced the self-degradation and mineralization of various organics, including phenolics (bisphenol A and phenol), antibiotics (ibuprofen and tetracycline), and dyes (methylene bule and rhodamine B). Compared with traditional Fe(II)-PS and Fe(II)–H2O2 systems, the organic-Fe(III)-PS-TiO2-Vis process requires a lower dosage of iron salt. The effective pH range has been broadened to neutral conditions due to effective prevention of Fe(III) precipitation and rapid circulation of Fe(III)/Fe(II). The comprehensive mechanistic study indicated that a synergistic effect was generated via Fe(III) reduction, PS activation, ROS generation and organic decomposition, resulting in sustainable and excellent catalytic performance of this novel Fenton-like process. Further, the results of cycling experiments and tests involving real industrial wastewater highlight the enormous potential of the proposed LMCT-mediated heterogeneous Fenton-like process in environmental remediation." @default.
• W4280636120 created "2022-05-22" @default.
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• W4280636120 date "2022-10-01" @default.
• W4280636120 modified "2023-10-18" @default.
• W4280636120 title "Efficient Fe(III) reduction and persulfate activation induced by ligand-to-metal charge transfer under visible light enhances degradation of organics" @default.
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• W4280636120 doi "https://doi.org/10.1016/j.cej.2022.137052" @default.
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