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• W4281489269 startingPage "4747" @default.
• W4281489269 abstract "The detection of intermediate species and the correlation of their ultrafast dynamics with the morphology and electronic structure of a surface is crucial to fully understand and control heterogeneous photoinduced and photocatalytic reactions. In this work, the ultrafast photodissociation dynamics of CH3Br molecules adsorbed on variable-size Au clusters on MgO/Mo(100) is investigated by monitoring the CH3+ transient evolution using a pump-probe technique in conjunction with surface mass spectrometry. Furthermore, extreme-UV photoemission spectroscopy in combination with theoretical calculations is employed to study the electronic structure of the Au clusters on MgO/Mo(100). Changes in the ultrafast dynamics of the CH3+ fragment are correlated with the electronic structure of Au as it evolves from monomers to small nonmetallic clusters to larger nanoparticles with a metallic character. This work provides a new avenue to a detailed understanding of how surface-photoinduced chemical reactions are influenced by the composition and electronic structure of the surface." @default.
• W4281489269 created "2022-05-26" @default.
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• W4281489269 date "2022-05-25" @default.
• W4281489269 modified "2023-09-25" @default.
• W4281489269 title "Nonmetal-to-Metal Transition of Magnesia Supported Au Clusters Affects the Ultrafast Dissociation Dynamics of Adsorbed CH₃Br Molecules" @default.
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• W4281489269 doi "https://doi.org/10.1021/acs.jpclett.2c00968" @default.
• W4281489269 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35612537" @default.
• W4281489269 hasPublicationYear "2022" @default.
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