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- W4281567002 abstract "Among multitudinous development methods of the active sites of MOFs, the encapsulation method is widely used. However, metal ions with excellent catalytic performance are not suitable for being directly encapsulated in MOFs. Because metal ions are much smaller than the pore sizes of MOFs, they will move in and out of the channels of MOFs haphazardly rather than being stably loaded in the channels like that of enzymes and metal nanoparticles. Here, to solve the above-mentioned problem, the metal ion Pd(II) was introduced into the single-chain polymer nanoparticles (SCNP) to form Pd(II) cross-linked SCNP (Pd-SCNP). A bifunctional heterogeneous catalyst [email protected] was prepared by introducing Pd-SCNP and chiral proline into the channels and on the Zr-clusters of DUT-67, respectively. The catalyst displayed excellent enantioselectivity and good coupling performance in Suzuki coupling/asymmetric aldol sequential reactions. Besides, [email protected] still retained good catalytic activity within three cycles of reuse." @default.
- W4281567002 created "2022-05-27" @default.
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- W4281567002 date "2022-07-01" @default.
- W4281567002 modified "2023-10-01" @default.
- W4281567002 title "Single-chain polymer nanoparticles-encapsulated chiral bifunctional metal-organic frameworks for asymmetric sequential reactions" @default.
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- W4281567002 doi "https://doi.org/10.1016/j.inoche.2022.109577" @default.
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