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- W4281567888 abstract "The existence of long-range magnetic order in low-dimensional magnetic systems, such as the quasi-two-dimensional van der Waals (vdW) magnets, has attracted intensive studies of new physical phenomena. The vdW Fe_{N}GeTe_{2} (N=3, 4, 5; FGT) family is exceptional, owing to its vast tunability of magnetic properties. In particular, a ferromagnetic ordering temperature (T_{C}) above room temperature at N=5 (F5GT) is observed. Here, our study shows that, by nickel (Ni) substitution of iron in F5GT, a record high T_{C}=478(6) K is achieved. Importantly, pervasive, beyond room-temperature ferromagnetism exists in almost the entire doping range of the phase diagram of Ni-F5GT. We argue that this striking observation in Ni-F5GT can be possibly due to several contributing factors, including increased 3D magnetic couplings due to the structural alterations." @default.
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- W4281567888 date "2022-05-26" @default.
- W4281567888 modified "2023-10-16" @default.
- W4281567888 title "Pervasive beyond Room-Temperature Ferromagnetism in a Doped van der Waals Magnet" @default.
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- W4281567888 doi "https://doi.org/10.1103/physrevlett.128.217203" @default.
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