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- W4281608258 abstract "A single quantum dot (QD) strongly coupled with a plasmonic nanoparticle yields a promising qubit for scalable solid-state quantum information processing at room temperature. However, realizing such a strong coupling remains challenging due to the difficulty of spatial overlap of the QD excitons with the plasmonic electric fields (EFs). Here, by using a transmission electron microscope we demonstrate for the first time that this overlap can be realized by integrating a deterministic single QD with a single Au nanorod. When a wedge nanogap cavity consisting of them and the substrate is constructed, the plasmonic EFs can be more effectively dragged and highly confined in the QD's nanoshell where the excitons mainly reside. With these advantages, we observed the largest spectral Rabi splitting (reported so far) of ∼234 meV for a single QD strong coupling with plasmons. Our work opens a pathway to the massive construction of room-temperature strong coupling solid qubits." @default.
- W4281608258 created "2022-06-12" @default.
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- W4281608258 date "2022-05-31" @default.
- W4281608258 modified "2023-10-16" @default.
- W4281608258 title "Room-Temperature Strong Coupling Between a Single Quantum Dot and a Single Plasmonic Nanoparticle" @default.
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- W4281608258 doi "https://doi.org/10.1021/acs.nanolett.2c00606" @default.
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