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• W4281618504 abstract "A novel Zn-Fe flow battery featuring an Fe3+ reduction reaction (Fe3+ RR)-coupled zinc oxidation, and an Fe2+ oxidation reaction (Fe2+ OR)-coupled hydrogen evolution reaction (HER) system as well, was established. This battery is capable of driving two Fe2+ OR-coupled HER systems in series based on the above Fe2+ /Fe3+ cycling, for efficient self-powered hydrogen evolution. Meanwhile, this Fe2+ /Fe3+ cycling enables the preparation of a multifunctional catalyst, Pt-3@SXNS (siloxene nanosheet), by the Fe2+ OR-promoted dispersion of Pt nanoparticles on SXNS; alternatively, this support could be obtained by Fe3+ RR-assisted exfoliation using Fe3+ from the anolyte of Fe2+ OR-coupled HER. The Pt-3@SXNS catalyst exhibits excellent catalytic activities toward Fe3+ RR in the Zn-Fe flow battery, HER, and Fe2+ OR in the electrolyzer, which is attributed to the strong electronic interaction between Pt and Si. This work offers a new strategy for energy storage and low-cost hydrogen production from acidic wastewater." @default.
• W4281618504 created "2022-06-13" @default.
• W4281618504 creator A5002463749 @default.
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• W4281618504 date "2022-06-23" @default.
• W4281618504 modified "2023-10-15" @default.
• W4281618504 title "Fe²⁺/Fe³⁺ Cycling for Coupling Self‐Powered Hydrogen Evolution and Preparation of Electrode Catalysts" @default.
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• W4281618504 doi "https://doi.org/10.1002/anie.202207226" @default.
• W4281618504 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35638129" @default.
• W4281618504 hasPublicationYear "2022" @default.
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