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- W4281653759 abstract "The design of composite photocatalytic materials is essential for efficient photocatalytic hydrogen production. In the present work, we have successfully designed a simple synthetic process to ultrathin ReSe2 nanosheets using an ultrasound-assisted liquid-phase synthetic route through self-assembling ReSe2 onto g-C3N4 (shortened as g-C3N4/ReSe2 nanosheets) to improve photocatalytic performance. Based on density functional theory (DFT) estimation along with experimental characterization, it is found that the integrated heterojunction-like ultrathin g-C3N4/ReSe2 nanosheets possess more edge active sites, enhanced electron transfer efficiency and conductivities, which significantly accelerates the dissociation and migration of photogenerated electron-hole pairs. Meanwhile, selenium vacancies could be introduced into nanosheets via controlling the synthetic procedure with a reduced Se source that will favor to enhance the photocatalytic efficiency. The ultrathin g-C3N4/ReSe2 heterojunction with Se vacancies performed highly improved photocatalytic hydrogen production. In typical, the H2 production of the g-C3N4/ReSe2 nanosheets under visible light is 1055.50 μmol g−1 h−1, which is 21 times higher than that of bare g-C3N4, indicating that it overcomes the high charge complexation rate of g-C3N4. These results do not only provide insight into the application of two-dimensional ReSe2 nanosheets in photocatalysis, but also open up new avenues for the rational design of two-dimensional hybrid materials in solar energy conversion." @default.
- W4281653759 created "2022-06-13" @default.
- W4281653759 creator A5015826633 @default.
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- W4281653759 creator A5067394066 @default.
- W4281653759 date "2022-10-01" @default.
- W4281653759 modified "2023-10-17" @default.
- W4281653759 title "Enhanced solar-driven hydrogen evolution over ultrathin g-C3N4/ReSe2 heterojunction-like nanosheets with surface selenium vacancies" @default.
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- W4281653759 doi "https://doi.org/10.1016/j.jallcom.2022.165786" @default.
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