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- W4281661271 abstract "Fixed-bed reactors employed within Power-to-X technologies are expected to be subject to volatile process feeds, in order to minimize intermediate buffer or storage systems. In this context, catalyst particles with an inert shell have proven suitable to prevent reactor runaway and severe temperature excursion at various loads and during load-changes, while still allowing for high reactor space-time yields. The aim of this work is to determine how much active catalyst mass can be saved by multi-period design optimization of methanation reactors with one, two, and infinite fixed-bed segments. Our results show that the amount of active mass, which can be saved with a single fixed-bed segment, is negligible. If more than one fixed-bed segment is considered, up to 45.2 % can be saved at the expense of a more complex dynamic reactor behavior. In the worst case, severe temperature excursions during transient scenarios might occur, which is not the case, if only a single fixed-bed segment is considered." @default.
- W4281661271 created "2022-06-13" @default.
- W4281661271 date "2022-06-01" @default.
- W4281661271 modified "2023-09-25" @default.
- W4281661271 title "Design approved for world’s first methane oxidation catalyst system" @default.
- W4281661271 doi "https://doi.org/10.1016/j.focat.2022.05.035" @default.
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