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- W4281689938 abstract "Due to the assets such as adequate discharge capacity and rational cost, LiNi0.8Co0.15Al0.05O2(NCA), a high-nickel ternary layered oxide, is regarded to be a favorable cathode contender for lithium-ion batteries. However, the superior commercial application is restricted by the surface residual alkaline lithium salt (LiOH or/and Li2CO3) of nickel-rich cathode materials, which will expedite the disintegration of the structure and the engendering of gas (CO2). Therefore, in this paper, we devise and fabricate a Y(PO3)3modified LiNi0.8Co0.15Al0.05O2(NCA), intending to optimize the surface residual alkaline lithium salt (antecedent deportation of H2O and CO2) while forming anin situtriple composite Li-ion conductor coating (Y(PO3)3-Li3PO4-YPO4) to enhance the electrochemical behavior. Under this method, the 2 mol% Y(PO3)3modified NCA electrode reveals exceptional rate capability (5 C/156.3 mAh g-1) and extraordinary cycle stability after 200 cycles (2 C/88.3%), whereas the original sample is only 5 C/123.1 mAh g-1and 2 C/71.2% after 200 cycles. Conspicuously, even under the draconian circumstances of the high temperature and the high rate at 55 °C/1 C, the 2 mol% Y(PO3)3modified NCA electrode sustains a high reversible capacity, with an admirable capacity retention rate of 89.4% after 100 cycles. These contented results signify that the surface remodeling tactic presents a viable scheme for ameliorating high-nickel materials' performance and appropriateness." @default.
- W4281689938 created "2022-06-13" @default.
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- W4281689938 date "2022-06-20" @default.
- W4281689938 modified "2023-09-27" @default.
- W4281689938 title "Face-lifting the surface of LiNi<sub>0.8</sub>Co<sub>0.15</sub>Al<sub>0.05</sub>O<sub>2</sub> cathode via Y(PO<sub>3</sub>)<sub>3</sub> to form an in situ triple composite Li-ion conductor coating layer with the enhanced electrochemical performance" @default.
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- W4281689938 doi "https://doi.org/10.1088/1361-6528/ac7577" @default.
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