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- W4281718178 abstract "2,3-Dichloro-5,6-dicyano-1,4-benzoquinone (DDQ) is a commonly known oxidant. Herein, we report that DDQ can be used to synthesize 1,2-disubstituted benzimidazoles and quinazolin-4(3 H )-ones via the intra- and intermolecular C–N coupling reaction under solvent-free mechanochemical (ball milling) conditions. In the presence of DDQ, the intramolecular C(sp 2 )–H amidation of N -(2-(arylideneamino)phenyl)- p -toluenesulfonamides leads to 1,2-disubstituted benzimidazoles and the one-pot coupling of 2-aminobenzamides with aryl/alkyl aldehydes resulted in substituted quinazolin-4(3 H )-one derivatives in high yields." @default.
- W4281718178 created "2022-06-13" @default.
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- W4281718178 date "2022-06-01" @default.
- W4281718178 modified "2023-10-18" @default.
- W4281718178 title "DDQ in mechanochemical C–N coupling reactions" @default.
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- W4281718178 doi "https://doi.org/10.3762/bjoc.18.64" @default.
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