Matches in SemOpenAlex for { <https://semopenalex.org/work/W4281738293> ?p ?o ?g. }
- W4281738293 endingPage "25489" @default.
- W4281738293 startingPage "25478" @default.
- W4281738293 abstract "The electrocatalytic reduction of nitrobenzene to aniline normally faces high overpotential and poor selectivity because of its six-electron redox nature. Herein, a Ag nanoparticles/laser-induced-graphene (LIG) heterointerface was fabricated on polyimide films and employed as an electrode material for an efficient nitrobenzene reduction reaction (NBRR) via a one-step laser direct writing technology. The first-principles calculations reveal that Ag/LIG shows the lowest activation barriers for the NBRR, which could be attributed to the optimum adsorption of the H atom realized by the appropriate interaction between Ag/LIG heterointerfaces and nitrobenzene. As a result, the overpotential of the NBRR is reduced by 217 mV after silver loading, and Ag/LIG shows a high aniline selectivity of 93%. Furthermore, an electrochemical reduction of nitrobenzene in tandem with an electrochemical oxidative polymerization of aniline was designed to serve as an alternative method to remove nitrobenzene from the aqueous solution. This strategy highlights the significance of heterointerfaces for efficient electrocatalysts, which may stimulate the development of novel electrocatalysts to boost the electrocatalytic activity." @default.
- W4281738293 created "2022-06-13" @default.
- W4281738293 creator A5006258018 @default.
- W4281738293 creator A5019691378 @default.
- W4281738293 creator A5044617186 @default.
- W4281738293 creator A5047101206 @default.
- W4281738293 creator A5069491797 @default.
- W4281738293 creator A5076784728 @default.
- W4281738293 creator A5077352796 @default.
- W4281738293 creator A5079020384 @default.
- W4281738293 creator A5090484465 @default.
- W4281738293 date "2022-05-30" @default.
- W4281738293 modified "2023-10-18" @default.
- W4281738293 title "Asymmetric Activation of the Nitro Group over a Ag/Graphene Heterointerface to Boost Highly Selective Electrocatalytic Reduction of Nitrobenzene" @default.
- W4281738293 cites W1981368803 @default.
- W4281738293 cites W1981482501 @default.
- W4281738293 cites W1989651443 @default.
- W4281738293 cites W1990206559 @default.
- W4281738293 cites W2026782811 @default.
- W4281738293 cites W2040407169 @default.
- W4281738293 cites W2045912757 @default.
- W4281738293 cites W2049326012 @default.
- W4281738293 cites W2065020992 @default.
- W4281738293 cites W2067251097 @default.
- W4281738293 cites W2073494397 @default.
- W4281738293 cites W2078837022 @default.
- W4281738293 cites W2078872586 @default.
- W4281738293 cites W2091183167 @default.
- W4281738293 cites W2120145199 @default.
- W4281738293 cites W2136334331 @default.
- W4281738293 cites W2318286541 @default.
- W4281738293 cites W2344366684 @default.
- W4281738293 cites W2465567597 @default.
- W4281738293 cites W2555600492 @default.
- W4281738293 cites W2740339667 @default.
- W4281738293 cites W2747318948 @default.
- W4281738293 cites W2761480616 @default.
- W4281738293 cites W2795940383 @default.
- W4281738293 cites W2808689666 @default.
- W4281738293 cites W2883556353 @default.
- W4281738293 cites W2883749332 @default.
- W4281738293 cites W2888587442 @default.
- W4281738293 cites W2902566206 @default.
- W4281738293 cites W2907375416 @default.
- W4281738293 cites W2908880033 @default.
- W4281738293 cites W2928096726 @default.
- W4281738293 cites W2940515244 @default.
- W4281738293 cites W2947809273 @default.
- W4281738293 cites W2948831591 @default.
- W4281738293 cites W2957091067 @default.
- W4281738293 cites W2969762738 @default.
- W4281738293 cites W2978479372 @default.
- W4281738293 cites W2988111892 @default.
- W4281738293 cites W3005568347 @default.
- W4281738293 cites W3019038224 @default.
- W4281738293 cites W3026566923 @default.
- W4281738293 cites W3049468435 @default.
- W4281738293 cites W3149168366 @default.
- W4281738293 cites W3159084225 @default.
- W4281738293 cites W3161551980 @default.
- W4281738293 cites W3164790702 @default.
- W4281738293 cites W3185157829 @default.
- W4281738293 cites W3190064887 @default.
- W4281738293 cites W4210809232 @default.
- W4281738293 doi "https://doi.org/10.1021/acsami.2c04533" @default.
- W4281738293 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35634976" @default.
- W4281738293 hasPublicationYear "2022" @default.
- W4281738293 type Work @default.
- W4281738293 citedByCount "9" @default.
- W4281738293 countsByYear W42817382932022 @default.
- W4281738293 countsByYear W42817382932023 @default.
- W4281738293 crossrefType "journal-article" @default.
- W4281738293 hasAuthorship W4281738293A5006258018 @default.
- W4281738293 hasAuthorship W4281738293A5019691378 @default.
- W4281738293 hasAuthorship W4281738293A5044617186 @default.
- W4281738293 hasAuthorship W4281738293A5047101206 @default.
- W4281738293 hasAuthorship W4281738293A5069491797 @default.
- W4281738293 hasAuthorship W4281738293A5076784728 @default.
- W4281738293 hasAuthorship W4281738293A5077352796 @default.
- W4281738293 hasAuthorship W4281738293A5079020384 @default.
- W4281738293 hasAuthorship W4281738293A5090484465 @default.
- W4281738293 hasConcept C118792377 @default.
- W4281738293 hasConcept C147789679 @default.
- W4281738293 hasConcept C161790260 @default.
- W4281738293 hasConcept C171250308 @default.
- W4281738293 hasConcept C17525397 @default.
- W4281738293 hasConcept C178790620 @default.
- W4281738293 hasConcept C179104552 @default.
- W4281738293 hasConcept C185592680 @default.
- W4281738293 hasConcept C186460083 @default.
- W4281738293 hasConcept C191897082 @default.
- W4281738293 hasConcept C192562407 @default.
- W4281738293 hasConcept C2779244968 @default.
- W4281738293 hasConcept C2780809723 @default.
- W4281738293 hasConcept C30080830 @default.
- W4281738293 hasConcept C52859227 @default.
- W4281738293 hasConcept C55904794 @default.
- W4281738293 hasConcept C75473681 @default.