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• W4281741244 abstract "Abstract Iron‐doped tin oxide (Sn 0.9 Fe 0.1 O 2 ), and specifically carbon‐coated Sn 0.9 Fe 0.1 O 2 (Sn 0.9 Fe 0.1 O 2 ‐C) provides high reversible capacity and a reasonably low de‐/lithiation potential owing to the combined conversion and alloying mechanism. The initial (quasi‐)amorphization during the first lithiation, however, renders an in‐depth understanding of the reaction mechanism challenging. Herein, a comprehensive investigation via a set of highly complementary characterization techniques is reported, including operando X‐ray diffraction, ex situ 119 Sn and 57 Fe Mössbauer spectroscopy, ex situ 7 Li NMR spectroscopy, operando isothermal microcalorimetry (IMC) of Li‖Sn 0.9 Fe 0.1 O 2 ‐C coin cells, and electrochemical microcalorimetry of single Sn 0.9 Fe 0.1 O 2 ‐C electrodes. The combination of these advanced techniques allows for detailed insights into the lithiation and delithiation mechanism and the potential determining processes, despite the (quasi‐) amorphous nature of the active material after the initial lithiation." @default.
• W4281741244 created "2022-06-13" @default.
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• W4281741244 date "2022-06-01" @default.
• W4281741244 modified "2023-10-02" @default.
• W4281741244 title "Comprehensive Approach to Investigate the De‐/Lithiation Mechanism of Fe‐Doped SnO₂ as Lithium‐Ion Anode Material" @default.
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• W4281741244 doi "https://doi.org/10.1002/adsu.202200102" @default.
• W4281741244 hasPublicationYear "2022" @default.
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