Matches in SemOpenAlex for { <https://semopenalex.org/work/W4281752016> ?p ?o ?g. }
- W4281752016 endingPage "121210" @default.
- W4281752016 startingPage "121210" @default.
- W4281752016 abstract "• Solar light-assisted peroxymonosulfate activation as an eco-friendly means for tetracycline degradation. • A g-C 3 N 4 -based S-scheme heterostructure (g-C 3 N 4 /Ag/AgNCO) fabricated via a facile approach. • Enhanced light absorption, charge separation/transport account for promising tetracycline degradation efficiency. • The quenching/ESR investigations reveal the significance of active species being h + > SO 4 •− ∼ • O 2 – > 1 O 2 > • OH. • The reaction routes, degradation intermediates, and toxicity assessment of TC explored in detail. Photo-assisted peroxymonosulfate (PMS) activation process is emerging as an effective and eco-friendly technology for sewage purification. Herein, a g-C 3 N 4 -based S-scheme heterostructure (g-C 3 N 4 /Ag/AgNCO) was fabricated by a facile chemical-deposition and photo-reduction method. Because of intensive hetero-interface contact and synergistic effect between g-C 3 N 4 and Ag/AgNCO, the assembled heterojunction exhibits enhanced light absorption, rapid charge separation/transport and impressive catalytic performance. Tetracycline (TC) degradation efficiency of 98% with a rate constant of 0.2995 min −1 can be accomplished over 40%-g-C 3 N 4 /Ag/AgNCO/PMS/light system within 12 min, 3.05 and 4.86 times better than that obtained over g-C 3 N 4 /PMS/light and AgNCO/PMS/light system, respectively. The quenching/ESR investigation suggested that the active species function syngenetically in TC degradation and the significance follows the order of h + > SO 4 •− ∼ • O 2 – > 1 O 2 > • OH. The cyclic test proved the excellent stability of the current catalyst system. The involved degradation routes, intermediates, and toxicity assessment have been studied in detail. The current research may serve as a versatile tactic for designing the g-C 3 N 4 -based functionalized catalytic material for wastewater purification through the photocatalysis/sulfate-mediated advanced treatment process." @default.
- W4281752016 created "2022-06-13" @default.
- W4281752016 creator A5030164210 @default.
- W4281752016 creator A5032477554 @default.
- W4281752016 creator A5055808596 @default.
- W4281752016 creator A5056510468 @default.
- W4281752016 creator A5066543327 @default.
- W4281752016 date "2022-09-01" @default.
- W4281752016 modified "2023-10-02" @default.
- W4281752016 title "S-scheme heterojunction g-C3N4/Ag/AgNCO for efficient tetracycline removal in a photo-assisted peroxymonosulfate system" @default.
- W4281752016 cites W1870103209 @default.
- W4281752016 cites W2125999138 @default.
- W4281752016 cites W2300532068 @default.
- W4281752016 cites W2554515147 @default.
- W4281752016 cites W2586685392 @default.
- W4281752016 cites W2768496904 @default.
- W4281752016 cites W2781765495 @default.
- W4281752016 cites W2789007979 @default.
- W4281752016 cites W2797344004 @default.
- W4281752016 cites W2800458938 @default.
- W4281752016 cites W2870035251 @default.
- W4281752016 cites W2884063536 @default.
- W4281752016 cites W2888504759 @default.
- W4281752016 cites W2889604339 @default.
- W4281752016 cites W2891629467 @default.
- W4281752016 cites W2900453087 @default.
- W4281752016 cites W2900490912 @default.
- W4281752016 cites W2904727058 @default.
- W4281752016 cites W2921826877 @default.
- W4281752016 cites W2936422568 @default.
- W4281752016 cites W2946141434 @default.
- W4281752016 cites W2946180626 @default.
- W4281752016 cites W2972761974 @default.
- W4281752016 cites W2995789837 @default.
- W4281752016 cites W3012459038 @default.
- W4281752016 cites W3013909924 @default.
- W4281752016 cites W3017333505 @default.
- W4281752016 cites W3033852833 @default.
- W4281752016 cites W3036541186 @default.
- W4281752016 cites W3040817382 @default.
- W4281752016 cites W3092691791 @default.
- W4281752016 cites W3094024123 @default.
- W4281752016 cites W3094074828 @default.
- W4281752016 cites W3096008438 @default.
- W4281752016 cites W3104998505 @default.
- W4281752016 cites W3112256234 @default.
- W4281752016 cites W3116063741 @default.
- W4281752016 cites W3119755811 @default.
- W4281752016 cites W3127209431 @default.
- W4281752016 cites W3133230630 @default.
- W4281752016 cites W3136522234 @default.
- W4281752016 cites W3156161785 @default.
- W4281752016 cites W3157709067 @default.
- W4281752016 cites W3157816002 @default.
- W4281752016 cites W3161584275 @default.
- W4281752016 cites W3161641145 @default.
- W4281752016 cites W3162518132 @default.
- W4281752016 cites W3162587953 @default.
- W4281752016 cites W3163103490 @default.
- W4281752016 cites W3163299845 @default.
- W4281752016 cites W3172481630 @default.
- W4281752016 cites W3177541978 @default.
- W4281752016 cites W3177993836 @default.
- W4281752016 cites W3178857260 @default.
- W4281752016 cites W3182941230 @default.
- W4281752016 cites W3183781074 @default.
- W4281752016 cites W3184197505 @default.
- W4281752016 cites W3194190410 @default.
- W4281752016 cites W3198619623 @default.
- W4281752016 cites W3200747286 @default.
- W4281752016 cites W3200879458 @default.
- W4281752016 cites W3202462003 @default.
- W4281752016 cites W3202501103 @default.
- W4281752016 cites W3203428574 @default.
- W4281752016 cites W3204285738 @default.
- W4281752016 cites W4220697366 @default.
- W4281752016 doi "https://doi.org/10.1016/j.seppur.2022.121210" @default.
- W4281752016 hasPublicationYear "2022" @default.
- W4281752016 type Work @default.
- W4281752016 citedByCount "14" @default.
- W4281752016 countsByYear W42817520162022 @default.
- W4281752016 countsByYear W42817520162023 @default.
- W4281752016 crossrefType "journal-article" @default.
- W4281752016 hasAuthorship W4281752016A5030164210 @default.
- W4281752016 hasAuthorship W4281752016A5032477554 @default.
- W4281752016 hasAuthorship W4281752016A5055808596 @default.
- W4281752016 hasAuthorship W4281752016A5056510468 @default.
- W4281752016 hasAuthorship W4281752016A5066543327 @default.
- W4281752016 hasConcept C127413603 @default.
- W4281752016 hasConcept C134306372 @default.
- W4281752016 hasConcept C13965031 @default.
- W4281752016 hasConcept C161790260 @default.
- W4281752016 hasConcept C178790620 @default.
- W4281752016 hasConcept C185592680 @default.
- W4281752016 hasConcept C192562407 @default.
- W4281752016 hasConcept C2780923616 @default.
- W4281752016 hasConcept C33923547 @default.
- W4281752016 hasConcept C42360764 @default.