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- W4281768324 abstract "Nitrogen (N2 ) is an essential element for life, but kinetically stable N2 in the atmosphere needs to be reduced to biologically available forms as a nutrient for organisms. Abiotic nitrogen fixation is critical to the origin of life on the early Earth, which is due to lightning or mineral-based reduction. Here, synchrotron X-ray-induced silver nitrate formation on a silver copper (AgCu) thin-film is reported. Time-resolved X-ray diffraction measurements show that under intense X-ray exposure, initially formed silver oxides (AgOx) are quickly converted to silver nitrate (AgNO3 ). Interestingly, AgNO3 is first formed in its high-temperature phase with a space group of R3cH, which gradually transforms to the room temperature phase with a space group of Pbca under continuous X-ray irradiation. The result not only provides a new clue about the abiotic nitrogen reduction prior to life but also demonstrates a novel strategy of materials synthesis using synchrotron X-rays." @default.
- W4281768324 created "2022-06-13" @default.
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- W4281768324 date "2022-05-30" @default.
- W4281768324 modified "2023-09-23" @default.
- W4281768324 title "Synchrotron X‐Ray‐Driven Nitrogen Reduction on an AgCu Thin Film" @default.
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- W4281768324 doi "https://doi.org/10.1002/smll.202202720" @default.
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