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- W4281775132 abstract "We report the self-assembly of 2D double perovskite (BLA)2 CsAgBiBr7 (BLA=benzylammonium) on 3D Cs2 AgBiBr6 crystals, providing the first demonstration of polarization-sensitive photodetection using lead-free double perovskite heterocrystals (HCs). The (BLA)2 CsAgBiBr7 /Cs2 AgBiBr6 HC successfully combines the anisotropy of 2D double perovskites with the well-defined interface provided by heterogeneous integration. Driven by the built-in electric field in junction, photodetectors of HCs exhibit unique polarization dependence of zero-bias photocurrent with a large anisotropy ratio up to 9, which is 6 times amplified as compared to the pristine 2D (BLA)2 CsAgBiBr7 . More importantly, the present devices can remain polarization-sensitive with incident light intensity down to the nW cm-2 level. Our study on lead-free hybrid perovskite HCs marks a step toward establishing robust material foundations for fundamental scientific investigations and the development of optoelectronic devices." @default.
- W4281775132 created "2022-06-13" @default.
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- W4281775132 date "2022-07-04" @default.
- W4281775132 modified "2023-10-17" @default.
- W4281775132 title "Self‐Assembly of 2D Hybrid Double Perovskites on 3D Cs <sub>2</sub> AgBiBr <sub>6</sub> Crystals towards Ultrasensitive Detection of Weak Polarized Light" @default.
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- W4281775132 doi "https://doi.org/10.1002/anie.202205939" @default.
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