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- W4281855546 abstract "With increasing interest in hydrogen peroxide (H2O2) as an environmentally friendly oxidant for environmental remediation and a promising liquid fuel, we present herein a novel method for green and sustainable H2O2 production using versatile dopamine-based materials, demonstrating the conversion of H2O2 generation mechanism from a chemical to a photocatalytic process along with the structural transformation of dopamine to polydopamine. During the auto-oxidation of dopamine in the presence of oxygen, which involved the transition of catechol to hydroquinone groups and the ring closure of the amine group, H2O2 was chemically generated at a rate of 1.61 mmol g-1h−1 without an extra electron donor and additional energy sources. In contrast, self-polymerized polydopamine exhibited an effective photocatalytic H2O2 generation at a rate of 0.53 mmol g-1h−1 owing to its visible light absorptivity and semiconducting property. We anticipate that these unique properties of dopamine will provide a new class of organic-based, highly efficient solar-to-H2O2 conversion and sustainable energy systems in the future." @default.
- W4281855546 created "2022-06-13" @default.
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- W4281855546 date "2022-07-01" @default.
- W4281855546 modified "2023-10-02" @default.
- W4281855546 title "Sustainable hydrogen peroxide production based on dopamine through Janus-like mechanism transition from chemical to photocatalytic reactions" @default.
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- W4281855546 doi "https://doi.org/10.1016/j.jcat.2022.05.017" @default.
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