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- W4282000361 abstract "Synthesis of a potent inhibitor of bacterial protein synthesis, pleuromutilin, is described. Assembly of the critical cyclooctane fragment relies on an oxidative ring-expansion, and complete stereochemical relay in the synthetic sequence is enabled by the judicious choice of tactics. The requisite connectivity pattern of the perhydroindanone motif is rapidly established in a sequence of cycloaddition and radical cyclization events. Application of this strategy allows for preparation of the target natural product in 16 steps from commercially available material." @default.
- W4282000361 created "2022-06-13" @default.
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- W4282000361 date "2022-06-02" @default.
- W4282000361 modified "2023-09-25" @default.
- W4282000361 title "Synthesis of Pleuromutilin" @default.
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- W4282000361 doi "https://doi.org/10.1021/jacs.2c04708" @default.
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