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• W4282004393 endingPage "101051" @default.
• W4282004393 startingPage "101051" @default.
• W4282004393 abstract "Fossil fuel depletion and carbon dioxide (CO2) emission have driven worldwide research on alternative processes for the production of commodity chemicals. The high-efficiency catalysts can convert CO2 into high value-added products. Herein, the nanocable catalysts Pt–[email protected] were assembled using Pt–Ni alloy nanobead chains as core in UiO-67: a UiO-67 membrane growing along their outer edge. The nanocable structure can inhibit agglomeration and sintering of the nanobead chains to improve catalytic activity. The conversion of CO2 to CO reached 25.8% for Pt3[email protected] with a 13.2 nm-UiO-67 membrane, 12.3% for physically mixed Pt3Ni/UiO-67, and 10.8% for Pt3[email protected]52.1 with a 52.1 nm-UiO-67 membrane, demonstrating that an appropriate thickness of the UiO-67 membrane in Pt3[email protected] can enhance CO2 conversion to CO. Density functional theory calculations suggested that high CO2 conversion is associated with highly dispersed Ni. This work provides a feasible strategy for improving catalyst performance." @default.
• W4282004393 created "2022-06-13" @default.
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• W4282004393 date "2022-08-01" @default.
• W4282004393 modified "2023-10-16" @default.
• W4282004393 title "Pt–Ni alloy nanobead chains catalysts embedded in UiO-67 membrane for enhanced CO2 conversion to CO" @default.
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• W4282004393 doi "https://doi.org/10.1016/j.mtener.2022.101051" @default.
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