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• W4282034136 abstract "The rational electrolyte design with weak solvation is regarded as an effective way to regulate the electrolyte/electrode interface (SEI) that profoundly affects the performance of Li-metal batteries. Herein, we propose a newly developed siloxane-based weakly solvating electrolyte (SiBE) with contact ion pairs (CIPs) or aggregates (AGGs) dominating the solution structure, which enables the dendrite-free Li deposition and long cycle stability of Li-metal batteries. By altering the combination of Li salts, the SiBE leads to the formation of an inorganic anion-derived solid electrolyte interphase, which is highly stable and Li+-conductive. Based on SiBE, the Li||LiFePO4 (LFP) full cell can stably cycle for 1000 cycles at a 2C rate with a capacity retention of 76.9%. Even with a limited Li-metal anode, it can maintain a capacity retention of 80% after 110 cycles with a high average Coulombic efficiency of 99.8%. This work reveals that siloxane can be a promising solvent to obtain weakly solvating electrolytes, which opens a new avenue for SEI composition regulation of Li-metal batteries." @default.
• W4282034136 created "2022-06-13" @default.
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• W4282034136 date "2022-06-07" @default.
• W4282034136 modified "2023-10-16" @default.
• W4282034136 title "Designing Anion-Derived Solid Electrolyte Interphase in a Siloxane-Based Electrolyte for Lithium-Metal Batteries" @default.
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• W4282034136 doi "https://doi.org/10.1021/acsami.2c05098" @default.
• W4282034136 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35671243" @default.
• W4282034136 hasPublicationYear "2022" @default.
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