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• W4282831529 endingPage "7708" @default.
• W4282831529 startingPage "7699" @default.
• W4282831529 abstract "Fabrication of low-loading, noble-metal, stable, and high-performance metal catalysts remains a thorny issue. Herein, we demonstrate the successful formation of a hybrid nanostructure Pt/TiO2/SBA-15 catalyst (denoted as HNSC-P/T/S; Pt, 0.09%; TiO2, 10%) with satisfactory activity in the hydrogenation of para-chloronitrobenzene (p-CNB). The HNSC-P/T/S showed >99% conversion and a high selectivity of >98%, and the turnover frequency number (TOF) reached 66 766 h-1, which was impossible to achieve with Pt/TiO2 (denoted as P/T) or Pt/SBA-15 (denoted as P/S). The success of the catalytic activity of the HNSC-P/T/S mainly relies on its synergistic effect and special structure, which can fully develop the catalytic ability of Pt, thereby reducing the Pt loading in the noble-based catalyst. Furthermore, the HNSC-P/T/S could also achieve an excellent catalytic activity in the hydrogenation of other nitroarenes. Hence, this work proposes a direction to prepare a noble-based catalyst with a low loading of noble metals for diverse applications." @default.
• W4282831529 created "2022-06-15" @default.
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• W4282831529 date "2022-06-14" @default.
• W4282831529 modified "2023-10-17" @default.
• W4282831529 title "Hybrid Nanostructure Catalyst with Low Loading of Pt for the High-Efficiency Catalytic Hydrogenation of Chloronitrobenzene" @default.
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• W4282831529 doi "https://doi.org/10.1021/acs.langmuir.2c00531" @default.
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• W4282831529 hasPublicationYear "2022" @default.
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