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- W4282942017 abstract "Low-dimensional hybrid halide perovskite materials with self-trapped exciton (STE) emissions and anisotropic properties are highly attractive for their great potential in many applications. However, to date, reports on large one-dimensional (1D) perovskite single crystals have been limited. Here, centimeter-sized 1D single crystals of trimethylammonium lead iodide (TMAPbI3) with typical STE emission are synthesized by an antisolvent vapor-assisted crystallization method. Thermal quenching and antiquenching with a high relative sensitivity of photoluminescence (PL) are observed and studied via temperature-dependent photoluminescence spectroscopy. Further analysis indicates that the temperature-dependent PL behaviors are influenced by the self-trapping of the free exciton and the migrations between self-trapped excitons and intermediate nonradiative states. The TMAPbI3 single crystal also exhibits a linearly polarized emission and a large birefringence that is higher than those of commercial birefringent crystals. This 1D perovskite with high structural anisotropy has promise for applications in versatile optical- and luminescence-related fields." @default.
- W4282942017 created "2022-06-16" @default.
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- W4282942017 date "2022-06-09" @default.
- W4282942017 modified "2023-10-16" @default.
- W4282942017 title "Temperature-Dependent Luminescence and Anisotropic Optical Properties of Centimeter-Sized One-Dimensional Perovskite Trimethylammonium Lead Iodide Single Crystals" @default.
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- W4282942017 doi "https://doi.org/10.1021/acs.jpclett.2c01045" @default.
- W4282942017 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35679604" @default.
- W4282942017 hasPublicationYear "2022" @default.
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