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- W4282959094 abstract "Biopolymers are ideal candidates for the development of hydrogels for tissue engineering applications. However, chemical modifications are required to further improve their mechanical properties, in particular to cross-link them for long-lasting applications or biofabrication. Herein, we developed a novel gelatin-based hydrogel precursor, “GelmSi”. Gelatin was chosen as starting material because of its biocompatibility and bioactivity, favouring cell adhesion and migration. Alkoxysilane moieties were introduced in a controlled manner on the lysine side chains of gelatin to obtain a hybrid precursor which reacts in physiological conditions, forming covalent siloxane bonds and allowing the formation of a three-dimensional chemical network. On the contrary to unmodified gelatin, siloxane covalent network dramatically increases the stiffness and the thermal stability of the resulting gelatin-based hydrogel, making it suitable for cell encapsulation and cell culture. The biorthogonality and versatility of the GelmSi hybrid hydrogel unlock a broad range of gelatin-based bioengineering applications." @default.
- W4282959094 created "2022-06-17" @default.
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- W4282959094 date "2022-06-16" @default.
- W4282959094 modified "2023-10-15" @default.
- W4282959094 title "Gelatin modified with alkoxysilanes (GelmSi) forms hybrid hydrogels for bioengineering applications" @default.
- W4282959094 doi "https://doi.org/10.26434/chemrxiv-2022-lw81f" @default.
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