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• W4283009324 abstract "The rate-determining step of the oxygen evolution reaction based on a semiconductor photoanode is the formation of the OO bond. Herein, polyethylene glycol (PEG)-modified BiVO4 photoanodes are reported, in which protons can be transferred quickly due to the high proton conductivity of PEG, resulting in the acceleration of the OO bond formation rate. These are fully demonstrated by different kinetic isotope effect values. Moreover, the open-circuit voltage (Uoc ) further illustrates that PEG passivates the surface states and surface charge recombination is reduced. The composite photoanode can achieve a maximum photocurrent density of 3.64 mA cm-2 at 1.23 V compared to 1.04 mA cm-2 for pure BiVO4 , and an onset potential of 170 mV, which is a 230 mV negative shift compared to pure BiVO4 . This work provides a new strategy to accelerate water oxidation kinetics for photoanodes by speeding up the transfer of the proton and the OO bond formation rate." @default.
• W4283009324 created "2022-06-18" @default.
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• W4283009324 date "2022-06-16" @default.
• W4283009324 modified "2023-10-16" @default.
• W4283009324 title "Efficient Oxygen Evolution Reaction on Polyethylene Glycol‐Modified BiVO₄ Photoanode by Speeding up Proton Transfer" @default.
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• W4283009324 doi "https://doi.org/10.1002/smll.202201410" @default.
• W4283009324 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35708149" @default.
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