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- W4283067478 abstract "Membrane technology features inspiring excellence from numerous separation technologies for CO2 capture from post-combustion gas. Polyvinylamine (PVAm)-based facilitated transport membranes show significantly high separation performance, which has been proven promising for industrial scale-up. However, commercialized PVAm with low molecular weight and excessive crystallinity is not available to prepare high-performance membranes. Herein, the synthesis process of PVAm was optimized by regulating polymerization and acidic hydrolytic conditions. The membranes based on PVAm with a molecular weight of 154 kDa and crystallinity of 11.37% display high CO2 permeance of 726 GPU and CO2/N2 selectivity of 55 at a feed gas pressure of 0.50 MPa. Furthermore, we established a PVAm synthesis reactor with an annual PVAm solution (1%(mass)) capacity of over 7000 kg and realized the scaled-up manufacture of both PVAm and composite membranes." @default.
- W4283067478 created "2022-06-19" @default.
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- W4283067478 date "2022-10-01" @default.
- W4283067478 modified "2023-09-25" @default.
- W4283067478 title "Synthesis and optimization of high-performance amine-based polymer for CO2 separation" @default.
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- W4283067478 doi "https://doi.org/10.1016/j.cjche.2022.06.005" @default.
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