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• W4283072926 abstract "Single-atom active site catalysts have attracted significant attention in the field of photocatalytic CO 2 conversion. However, designing active sites for CO 2 reduction and H 2 O oxidation simultaneously on a photocatalyst and combining the corresponding half-reaction in a photocatalytic system is still difficult. Here, we synthesized a bimetallic single-atom active site photocatalyst with two compatible active centers of Mn and Co on carbon nitride (Mn 1 Co 1 /CN). Our experimental results and density functional theory calculations showed that the active center of Mn promotes H 2 O oxidation by accumulating photogenerated holes. In addition, the active center of Co promotes CO 2 activation by increasing the bond length and bond angle of CO 2 molecules. Benefiting from the synergistic effect of the atomic active centers, the synthesized Mn 1 Co 1 /CN exhibited a CO production rate of 47 μmol g -1 h -1 , which is significantly higher than that of the corresponding single-metal active site photocatalyst." @default.
• W4283072926 created "2022-06-19" @default.
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• W4283072926 date "2022-07-08" @default.
• W4283072926 modified "2023-09-25" @default.
• W4283072926 title "Carbon Nitride Photocatalysts with Integrated Oxidation and Reduction Atomic Active Centers for Improved CO ₂ Conversion" @default.
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• W4283072926 doi "https://doi.org/10.1002/ange.202206579" @default.
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