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• W4283080153 endingPage "121647" @default.
• W4283080153 startingPage "121647" @default.
• W4283080153 abstract "Glucose isomerization into fructose is a key process in industry for biomass valorization to produce value-added biofuels and biochemicals. Herein, considering the essential role of Lewis acid-base sites in proton transfer during glucose isomerization and hydrogen evolution process, a bifunctional polymeric red carbon nitride (PRCN) is rationally designed and fabricated by the salt-template-induced carbon incorporation strategy. The incorporation of carbon and potassium in the PRCN leads to the transient redistribution of photogenerated charges, acting as the electron-enriched Lewis base site and acid site for the deprotonation of O2-H and activation of aldehyde group of glucose, respectively. Besides, the interfacial Schottky junction boosts H 2 production under visible light irradiation. This work demonstrates the feasibility of biomass photorefinery with H 2 and value-added chemicals co-production under mild condition. Bifunctional polymeric red carbon nitride (PRCN) is rationally designed by introducing heteroatoms of carbon and potassium, acting as the electron-enriched Lewis base site and acid site for glucose isomerization. Hydrogen is simultaneously generated along with fructose production by the formation of Schottky junction with decoration of platinum nanoparticles. • Carbon incorporation in PRCN extended light absorbance to near-infrared region. • Heteroatomic carbon and potassium acted as Lewis base and acid site for glucose isomerization. • Schottky junction boosted H 2 co-production under visible light irradiation. • Electron-enriched C site reduced active H* transfer for glucose and promoted H 2 co-production." @default.
• W4283080153 created "2022-06-19" @default.
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• W4283080153 date "2022-11-01" @default.
• W4283080153 modified "2023-10-16" @default.
• W4283080153 title "Electron-enriched Lewis acid-base sites on red carbon nitride for simultaneous hydrogen production and glucose isomerization" @default.
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• W4283080153 doi "https://doi.org/10.1016/j.apcatb.2022.121647" @default.
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