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• W4283207009 abstract "• Proton irradiation effects in perovskite solar cells (PSCs) are investigated. • The PSCs exhibit superior resistance against proton irradiation. • Ionization irradiation leads to decomposition of the perovskite. • The Au electrode of the PSCs is finally exfoliated with increasing proton fluence. This study reports on the proton irradiation-induced property degradation in Cs 0.01 MA 0.01 FA 0.98 PbI 3 [MA = CH 3 NH 3 + , FA = CH(NH 2 ) 2 + ] perovskite films and solar cells (PSCs). Both 100 keV and 2 MeV protons are employed for irradiation. It is found that the threshold fluence for degradation of photovoltaic properties in PSCs is between 1 × 10 13 and 1 × 10 14 p/cm 2 for 100 keV proton irradiation, or between 1 × 10 14 and 2.2 × 10 15 p/cm 2 for 2 MeV proton irradiation. The degradation leads to a significant decrease in the short-circuit current; the open-circuit voltage is reduced to a less extent probably because of an increase in the electrical resistance across the interface between the perovskite and carrier transport layers. Irradiation-induced decomposition of CsMAFAPbI 3 to PbI 2 is observed due to the electronic energy deposition (radiolysis). With increasing proton fluence, the top Au electrode layer is finally exfoliated from the underlying spiro-OMeTAD layer, which could be attributed to the volume deformation of the spiro-OMeTAD induced by the accumulation of the gaseous products of perovskite decomposition." @default.
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• W4283207009 date "2022-09-01" @default.
• W4283207009 modified "2023-10-16" @default.
• W4283207009 title "Property degradation of mixed-cation perovskite films and solar cells irradiated with protons" @default.
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• W4283207009 doi "https://doi.org/10.1016/j.nimb.2022.06.012" @default.
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