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- W4283316534 abstract "The promotional effects of inert nitrides for metal catalysts in the electrolysis are rarely reported. Recently, we reported an efficient Ni-VN/NF (that NF represents Ni foam) composite by nitriding treatment of NiV-layered double hydroxides (NiV-LDH) precursor that was in-situ hydrothermal growth on nickel foam. The optimal Ni-VN/NF exhibited outstanding electrocatalytic performance for hydrogen evolution reaction (HER) with a small overpotential of 39 mV at 10 mA cm-2 and strong durability for 100 h without degradation. The optimized electronic structure and local charge density at the hetero-interface of Ni-VN, evidenced by both experiment and DFT results, were significantly modulated by the electron transfer from Ni to V-N bond at the interfaces, leading to moderate H* adsorption energy and diminished barrier for H2O dissociation, synergistically promoted basic HER. This work highlights the design principle of strong metal-nitride interactions for advanced HER catalysts." @default.
- W4283316534 created "2022-06-24" @default.
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- W4283316534 date "2022-11-01" @default.
- W4283316534 modified "2023-10-16" @default.
- W4283316534 title "Constructing Ni-VN interfaces with superior electrocatalytic activity for alkaline hydrogen evolution reaction" @default.
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- W4283316534 doi "https://doi.org/10.1016/j.jcis.2022.06.087" @default.
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