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• W4283380411 startingPage "1438" @default.
• W4283380411 abstract "Abstract Demonstrated herein is a synthetic strategy for M A M B M C ‐type heteronuclear metal‐string complexes (HMSC) in which the terminal metals can be tailored via a displacement reaction based on the relative coordination strength. The stability ruler Ni > Co > (Fe; Mn) > Cd > Cu is derived in this study. Accordingly, MPdM'(dpa) 4 Cl 2 (M ≠ M') can be obtained by the reaction of M' ion with MPdM(dpa) 4 Cl 2 if the relative stability is M' > M. Six M A M B M C ‐type HMSCs ( 2–7 ) with Pd at the central position are successfully synthesized. Unprecedented properties of metal strings, such as the structures, electrochemistry, and magnetism, are found. The static repulsion between terminal metals can dominate the metal–palladium distances. A shorter distance of Pd–M' at the opposite site can lengthen the Pd–M distance. The redox potentials of metal cores are influenced by this remote static repulsion. Besides, the nature of Cu with a weak spin‐exchange communication can induce the ferromagnetic coupling mediated by the central Pd in CuPdCo and CuPdNi HMSCs, and these are the first examples of ferromagnetism mediated by the central Pd metal among metal strings." @default.
• W4283380411 created "2022-06-25" @default.
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• W4283380411 date "2022-06-21" @default.
• W4283380411 modified "2023-09-27" @default.
• W4283380411 title "Metal replacement in the syntheses of <scp> M _A M _B M _C </scp> heterometallic metal‐string complexes: <scp>MPdM</scp> '(dpa) <scp> ₄ Cl ₂ </scp>" @default.
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• W4283380411 doi "https://doi.org/10.1002/jccs.202200154" @default.
• W4283380411 hasPublicationYear "2022" @default.
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