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• W4283399069 abstract "Zero-dimensional (0D) hybrid metal halides with unique compositional and structural tunability appear as an emerging class of luminescent materials, but near-infrared (NIR) emitters therein are largely unexplored to date. This study presents three novel 0D hybrid antimony chlorines with edge-sharing [Sb2 Cl8 ]2- dimers, showing unusual room-temperature broadband NIR emission with the maximum emission wavelength up to 1070 nm. Photoluminescence studies and density functional theory calculation demonstrate that the emissions originate from the highly localized excitons, and that the confined [Sb2 Cl8 ]2- dimers in these structures show low symmetry and a large degree of structural freedom. These hybrid antimony chlorines with [Sb2 Cl8 ]2- dimers expand the range of new NIR materials in 0D metal halides." @default.
• W4283399069 created "2022-06-25" @default.
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• W4283399069 date "2022-07-11" @default.
• W4283399069 modified "2023-10-09" @default.
• W4283399069 title "Highly Distorted Antimony(III) Chloride [Sb ₂ Cl ₈ ] ²⁻ Dimers for Near‐Infrared Luminescence up to 1070 nm" @default.
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• W4283399069 doi "https://doi.org/10.1002/anie.202208881" @default.
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