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• W4283662064 abstract "• Influences of heating-rates and experimental pressures were specifically evaluated. • High pressure would promote oxidation progress and weaken distillation with more heat formation. • Two distinct stages, LTO and HTO, were observed via the activation energy distribution curve. • Fitting between calculated and experimental curves indicated a reliable prediction. A better understanding of the influence factor investigation and oxidation behavior prediction for the crude oil could supply valuable insights into the reactivity of crude oil and feasibility of air injection process. In this study, non-isothermal oxidation experiments have been conducted via thermal analyses (thermogravimetry/differential scanning calorimetry/pressurized differential scanning calorimetry, TG/DSC/PDSC) with different heating rates (5, 10, and 15 °C/min) and experimental pressures (1, 3, and 5 MPa) in order to investigate the influences on oxidation behaviors, exothermic characteristics, and kinetic parameters of typical tight oil. In addition, the distributed activation energy method (DAEM) was employed to determine accurate kinetic parameters for whole oxidation process and to further predict the oxidation behavior with the reconstruction of TG and conversion curves. The results showed that, heating-rate increment would lead to inadequate oxidation process with more reaction occurrence in a shorter time. Inversely, more rapid heat release, higher exothermic peaks with lower temperature ranges were detected in PDSC curves, indicating high pressure in actual oil reservoir would strengthen the oxidation progress with more heat generation to enhance oil recovery. Then, based on specific activation energy distribution and DAEM, the calculated TG and conversion curves presented a satisfactory fitting relation with experimental data, demonstrating a reasonable prediction of oxidation behavior and kinetic characteristic for the crude oil under specific heating-rate. The understandings in this study not only provided new insights on the verification of obtained kinetic parameters, but also the accurate prediction of crude oil oxidation behavior." @default.
• W4283662064 created "2022-06-29" @default.
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• W4283662064 date "2022-10-01" @default.
• W4283662064 modified "2023-09-29" @default.
• W4283662064 title "New insights into the non-isothermal oxidation of tight oil: Experimental study and theoretical prediction" @default.
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• W4283662064 doi "https://doi.org/10.1016/j.fuel.2022.125011" @default.
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