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- W4283700866 abstract "An ultrastable and kinetically favorable interface is constructed between sulfide–poly(ethylene oxide) (PEO) composite solid electrolytes (CSEs) and lithium metal, via in situ formation of a solid electrolyte interphase (SEI) layer containing Li3PS4. A specially designed sulfide, lithium polysulfidophosphate (LPS), can distribute uniformly in the PEO matrix via a simple stirring process because of its complete solubility in acetonitrile solvent, which is advantageous for creating a homogeneous SEI layer. The CSE/Li interface with high Li+ transportation capability is stabilized quickly through in situ formation of a Li3PS4/Li2S/LiF layer via the reaction between LPS and lithium metal to inhibit lithium dendrite growth. A Li/Li symmetric cell with the LPS-integrated CSE exhibits constant and small CSE/Li resistance of 10 Ω cm2 during cycling, delivering stable cycling for 3475 h at a current density of 0.2 mA cm−2 and a high critical current density of 0.9 mA cm−2 at 60 °C. Impressive electrochemical performance is also demonstrated for LiFePO4/CSE/Li all-solid-state batteries with capacity of 127.6 mAh g−1 after 1000 cycles at 1 C." @default.
- W4283700866 created "2022-06-30" @default.
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- W4283700866 date "2022-07-21" @default.
- W4283700866 modified "2023-10-05" @default.
- W4283700866 title "Long‐Life Lithium‐Metal All‐Solid‐State Batteries and Stable Li Plating Enabled by In Situ Formation of Li <sub>3</sub> PS <sub>4</sub> in the SEI Layer" @default.
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- W4283700866 doi "https://doi.org/10.1002/adma.202203281" @default.
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