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- W4283713106 abstract "Glass containing magnetic nanocrystals are attractive for obtaining high magnetic and magneto-optical properties. In this study, for the first time, 10 nm cubic NiFe 2 O 4 (NFO) nanocrystals doped heavy metal oxide glasses were fabricated and the influence of NFO to glass structure, chemical bonds, Mössbauer spectra, magnetization and Faraday rotation was studied. X-ray diffraction, Raman and X-ray photoelectron spectra revealed the existence of multi-valence states of Fe/Ni ions, oxygen vacancies in cubic lattice and modifications on glass structure, which in turn adjusted the polarizability, oxygen packing density, Mössbauer spectra, magnetic property and magneto-optical behaviors. Through Mössbauer study, the increase of NFO amount enhanced the hyperfine field intensity of tetrahedral Fe 3+ ions at the expense of octahedral ones. NFO doped glasses exhibited ferromagnetic behavior whose M s and H c increased with the NFO amount due to the NCs size effect. Verdet constant and Faraday rotation angle were studied as function of wavelength, magnetic field, polarizer angle and NFO amount. 3%NFO glass exhibited significant enhancement in magnetization and Verdet constant of 91 rad/T.m at 633 nm which is 5-fold of host glass and superior than literatures. In addition, due to the nanoscale NCs, the thermal stability of obtained NFO glasses remained higher than 100 °C which is promising for photonics devices fabrication." @default.
- W4283713106 created "2022-06-30" @default.
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- W4283713106 date "2022-10-01" @default.
- W4283713106 modified "2023-10-06" @default.
- W4283713106 title "Spinel ferrites NiFe2O4 NCs enhanced Mössbauer spectra, magnetization and Faraday rotation of diamagnetic tellurite glasses" @default.
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- W4283713106 doi "https://doi.org/10.1016/j.ceramint.2022.06.292" @default.
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