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• W4283738439 endingPage "738" @default.
• W4283738439 startingPage "728" @default.
• W4283738439 abstract "Chemical reaction networks that transform out-of-equilibrium 'fuel' to 'waste' are the engines that power the biomolecular machinery of the cell. Inspired by such systems, autonomous artificial molecular machinery is being developed that functions by catalysing the decomposition of chemical fuels, exploiting kinetic asymmetry to harness energy released from the fuel-to-waste reaction to drive non-equilibrium structures and dynamics. Different aspects of chemical fuels profoundly influence their ability to power molecular machines. Here we consider the structure and properties of the fuels that biology has evolved and compare their features with those of the rudimentary synthetic chemical fuels that have so far been used to drive autonomous non-equilibrium molecular-level dynamics. We identify desirable, but context-specific, traits for chemical fuels together with challenges and opportunities for the design and invention of new chemical fuels to power synthetic molecular machinery and other dissipative nanoscale processes." @default.
• W4283738439 created "2022-07-02" @default.
• W4283738439 creator A5024470508 @default.
• W4283738439 creator A5052296013 @default.
• W4283738439 creator A5066396947 @default.
• W4283738439 date "2022-07-01" @default.
• W4283738439 modified "2023-10-14" @default.
• W4283738439 title "Chemical fuels for molecular machinery" @default.
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• W4283738439 doi "https://doi.org/10.1038/s41557-022-00970-9" @default.

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