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- W4283764897 abstract "Electrochemical nitrate reduction has become an appealing waste-to-wealth approach for sustainable NH3 synthesis owing to its mild operating conditions. However, developing catalysts with high activities and Faradaic efficiencies for this complicated eight-electron reaction is a great challenge. Herein, bismuth ferrite (BiFeO3) flakes, with a distorted perovskite-type structure, are demonstrated to be excellent catalysts for electrochemical NH3 synthesis via nitrate reduction, with a maximum Faradaic efficiency of 96.85%, NH3 yield of 90.45 mg h-1 mgcat-1, at -0.6 V vs. reversible hydrogen electrode. During the nitrate reduction reaction, the crystalline BiFeO3 rapidly converts into an amorphous phase, which is stable in the long term reaction. These results open a new window for rational design of more active and durable electrocatalysts." @default.
- W4283764897 created "2022-07-02" @default.
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- W4283764897 date "2022-07-01" @default.
- W4283764897 modified "2023-10-14" @default.
- W4283764897 title "Bismuth Ferrite as an Electrocatalyst for the Electrochemical Nitrate Reduction" @default.
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- W4283764897 doi "https://doi.org/10.1021/acs.nanolett.2c02026" @default.
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