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- W4284667986 abstract "Antimonene is a promising two-dimensional material predicted to host intriguing properties. Recent works have claimed the successful preparation of ensuremath{beta}-antimonene on noble metal surfaces, including Ag(111) and Cu(111). However, as scanning tunneling microscopy gives only the topographic information, the possibility of surface alloying for the claimed ensuremath{beta}-antimonene remains elusive. In this work, by scanning tunneling spectroscopy and in situ Raman spectroscopy measurements, we provide compelling evidence that the ``ensuremath{beta}-antimonenes'' on Ag(111) and Cu(111) reported in previous studies are both surface alloys, namely, ${mathrm{Ag}}_{2}mathrm{Sb}$ and ${mathrm{Cu}}_{2}mathrm{Sb}$. Thus, ensuremath{beta}-antimonene does not exist on these substrates. Instead, we find that ensuremath{alpha}-antimonene can be grown on both alloy surfaces, with different substrate-induced strain modulation effects. Our work not only clarifies the growth dynamics of Sb on Ag(111) and Cu(111) but also provides two model systems to realize ensuremath{alpha}-antimonene with tunable strains." @default.
- W4284667986 created "2022-07-08" @default.
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- W4284667986 date "2022-07-05" @default.
- W4284667986 modified "2023-10-17" @default.
- W4284667986 title "Absence of topological β-antimonene and growth of α-antimonene on noble metal Ag(111) and Cu(111) surfaces" @default.
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- W4284667986 doi "https://doi.org/10.1103/physrevmaterials.6.074002" @default.
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