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- W4284710020 abstract "Designing and synthesizing novel electrolyte and solid electrolyte interfaces (SEIs) are greatly desirable for improving the performance of lithium-ion batteries (LIBs). Taking into account the large surface area, chemical inertness, high lithium adsorption and surface modifiability, in this work, detonation nanodiamonds (NDs) with an average size of 5 nm were introduced to commercial LiPF6 electrolyte and a NDs-rich SEI was formed on graphitic anodes surface during charge–discharge processes. The NDs-rich SEIs have low interfacial resistance, fast ion transport and additional Li+ storage sites, which are favorable to improve the capacity and rate performance of LIBs. The half cells with ND-electrolyte exhibit capacities of ∼ 400 mA h g−1 at 5C (1C ∼ 372 mA h g−1) after 1000 cycles and ∼ 700 mA h g−1 at 0.2C after 100 cycles, which are nearly 2 times that for original electrolyte without NDs performed under the same processes. Further considering the compatibility with industrial processes, the strategy of forming SEIs consisting of NDs from electrolytes is helpful for fabricating high-performance LIBs with high capacity and stability for practical industrial applications." @default.
- W4284710020 created "2022-07-08" @default.
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- W4284710020 date "2022-10-01" @default.
- W4284710020 modified "2023-09-28" @default.
- W4284710020 title "Introducing nanodiamonds in electrolyte and SEI for highly improving performances of lithium-ion batteries" @default.
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- W4284710020 doi "https://doi.org/10.1016/j.apsusc.2022.154178" @default.
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