FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4284884818> ?p ?o ?g. }

• W4284884818 endingPage "8817" @default.
• W4284884818 startingPage "8805" @default.
• W4284884818 abstract "Abstract. Although knowledge of the physical state of aerosol particles is essential to understand atmospheric chemistry model and measurements, information on the viscosity and physical state of aerosol particles consisting of organic and inorganic salts is still rare. Herein, we quantified viscosities at 293 ± 1 K upon dehydration for the binary systems, sucrose–H2O and ammonium sulfate (AS)–H2O, and the ternary systems, sucrose–AS–H2O for organic-to-inorganic dry mass ratios (OIRs) = 4:1, 1:1, and 1:4 using bead-mobility and poke-and-flow techniques. Based on the viscosity value of the aerosol particles, we defined the physical states of the total aerosol particles studied in this work. For binary systems, the viscosity of sucrose–H2O particles gradually increased from ∼ 4 × 10−1 to > ∼ 1 × 108 Pa s when the relative humidity (RH) decreased from ∼ 81 % to ∼ 24 %, ranging from liquid to semisolid or solid state, which agrees with previous studies. The viscosity of AS–H2O particles remained in the liquid state (< 102 Pa s) for RH > ∼ 50 %, while for RH ≤∼ 50 %, the particles showed a viscosity of > ∼ 1 × 1012 Pa s, corresponding to a solid state. In case of the ternary systems, the viscosity of organic-rich particles (OIR = 4:1) gradually increased from ∼ 1 × 10−1 to ∼ 1 × 108 Pa s for a RH decrease from ∼ 81 % to ∼ 18 %, similar to the binary sucrose–H2O particles. This indicates that the sucrose–AS–H2O particles range from liquid to semisolid or solid across the RH. In the ternary particles for OIR = 1:1, the viscosities ranged from less than ∼ 1 × 102 for RH > 34 % to > ∼ 1 × 108 Pa s at ∼ 27 % RH. The viscosities correspond to liquid for RH > ∼ 34 %, semisolid for ∼ 34 % < RH < ∼ 27 %, and semisolid or solid for RH < ∼ 27 %. Compared to the organic-rich particles, in the inorganic-rich particles (OIR = 1:4), drastic enhancement in viscosity was observed as RH decreased; the viscosity increased by approximately 8 orders of magnitude during a decrease in RH from 43 % to 25 %, resulting in liquid to semisolid or solid in the RH range. Overall, all particles studied in this work were observed to exist as a liquid, semisolid, or solid depending on the RH. Furthermore, we compared the measured viscosities of ternary systems with OIRs of 4:1, 1:1, and 1:4 to the predicted viscosities using the Aerosol Inorganic–Organic Mixtures Functional groups Activity Coefficients Viscosity model (AIOMFAC-VISC) predictions with the Zdanovskii–Stokes–Robinson (ZSR) organic–inorganic mixing model, with excellent model–measurement agreement for all OIRs." @default.
• W4284884818 created "2022-07-09" @default.
• W4284884818 creator A5004408904 @default.
• W4284884818 creator A5009579319 @default.
• W4284884818 creator A5015204180 @default.
• W4284884818 creator A5047608068 @default.
• W4284884818 creator A5066965102 @default.
• W4284884818 creator A5067134431 @default.
• W4284884818 creator A5083941546 @default.
• W4284884818 creator A5090701573 @default.
• W4284884818 date "2022-07-08" @default.
• W4284884818 modified "2023-10-18" @default.
• W4284884818 title "Viscosity and physical state of sucrose mixed with ammonium sulfate droplets" @default.
• W4284884818 cites W1561878391 @default.
• W4284884818 cites W1614117239 @default.
• W4284884818 cites W1897778326 @default.
• W4284884818 cites W1952380628 @default.
• W4284884818 cites W1972590681 @default.
• W4284884818 cites W2001219782 @default.
• W4284884818 cites W2018296170 @default.
• W4284884818 cites W2025224855 @default.
• W4284884818 cites W2026094833 @default.
• W4284884818 cites W2031102891 @default.
• W4284884818 cites W2038135984 @default.
• W4284884818 cites W2039437298 @default.
• W4284884818 cites W2042175812 @default.
• W4284884818 cites W2047926788 @default.
• W4284884818 cites W2057253955 @default.
• W4284884818 cites W2059747079 @default.
• W4284884818 cites W2063168358 @default.
• W4284884818 cites W2080955504 @default.
• W4284884818 cites W2085914944 @default.
• W4284884818 cites W2088509007 @default.
• W4284884818 cites W2093674996 @default.
• W4284884818 cites W2094875133 @default.
• W4284884818 cites W2097531853 @default.
• W4284884818 cites W2102580742 @default.
• W4284884818 cites W2107520768 @default.
• W4284884818 cites W2123717816 @default.
• W4284884818 cites W2125740784 @default.
• W4284884818 cites W2126105726 @default.
• W4284884818 cites W2144608959 @default.
• W4284884818 cites W2144923407 @default.
• W4284884818 cites W2145798497 @default.
• W4284884818 cites W2148635929 @default.
• W4284884818 cites W2150164650 @default.
• W4284884818 cites W2153664297 @default.
• W4284884818 cites W2160853425 @default.
• W4284884818 cites W2161516788 @default.
• W4284884818 cites W2163922819 @default.
• W4284884818 cites W2164264901 @default.
• W4284884818 cites W2174234677 @default.
• W4284884818 cites W2180510201 @default.
• W4284884818 cites W2195744149 @default.
• W4284884818 cites W2299494704 @default.
• W4284884818 cites W2316803417 @default.
• W4284884818 cites W2318221707 @default.
• W4284884818 cites W2322823851 @default.
• W4284884818 cites W2518443403 @default.
• W4284884818 cites W2527292817 @default.
• W4284884818 cites W2531696317 @default.
• W4284884818 cites W2554285426 @default.
• W4284884818 cites W2591429460 @default.
• W4284884818 cites W2774523332 @default.
• W4284884818 cites W2901603400 @default.
• W4284884818 cites W2906748756 @default.
• W4284884818 cites W2913062554 @default.
• W4284884818 cites W2913365238 @default.
• W4284884818 cites W2942486523 @default.
• W4284884818 cites W2968831009 @default.
• W4284884818 cites W2990240899 @default.
• W4284884818 cites W2990437165 @default.
• W4284884818 cites W2999126468 @default.
• W4284884818 cites W3004424914 @default.
• W4284884818 cites W3015700659 @default.
• W4284884818 cites W3088275890 @default.
• W4284884818 cites W3103119442 @default.
• W4284884818 cites W3124841717 @default.
• W4284884818 cites W3130206662 @default.
• W4284884818 cites W3137781474 @default.
• W4284884818 cites W4210363077 @default.
• W4284884818 cites W4220890785 @default.
• W4284884818 cites W4224275887 @default.
• W4284884818 cites W4251688500 @default.
• W4284884818 doi "https://doi.org/10.5194/acp-22-8805-2022" @default.
• W4284884818 hasPublicationYear "2022" @default.
• W4284884818 type Work @default.
• W4284884818 citedByCount "7" @default.
• W4284884818 countsByYear W42848848182022 @default.
• W4284884818 countsByYear W42848848182023 @default.
• W4284884818 crossrefType "journal-article" @default.
• W4284884818 hasAuthorship W4284884818A5004408904 @default.
• W4284884818 hasAuthorship W4284884818A5009579319 @default.
• W4284884818 hasAuthorship W4284884818A5015204180 @default.
• W4284884818 hasAuthorship W4284884818A5047608068 @default.
• W4284884818 hasAuthorship W4284884818A5066965102 @default.
• W4284884818 hasAuthorship W4284884818A5067134431 @default.
• W4284884818 hasAuthorship W4284884818A5083941546 @default.

• next