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- W4284892193 abstract "The development of high-performance electrocatalysts for hydrogen evolution is essential and challenging. Recently, the engineering of nitride/carbide heterostructures with modulated heterointerfaces and strong synergistic effects has proven to be an effective strategy to improve catalytic performance. Herein, an innovative Mo2N/Mo2C heterostructure was synthesized by the ZIF-67 derivatization method as an efficient electrocatalyst for hydrogen generation. The optimal Mo2N/Mo2C-8 catalyst showed a low overpotential of 88.1 mV at 10 mA cm−2 (η10) and a small Tafel slope (68.5 mV dec−1) in 1 M KOH, as well as great stability. The synergistic effects from the unique nanohybridization of the Mo2N/Mo2C heterostructure greatly enhance the intrinsic catalytic activity, and the porous structure promotes mass transfer efficiency, thereby improving the HER performance. This finding provides an exciting opportunity to design advanced Mo-based HER electrocatalysts through interface engineering based on ZIF-67." @default.
- W4284892193 created "2022-07-09" @default.
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- W4284892193 date "2022-11-01" @default.
- W4284892193 modified "2023-09-30" @default.
- W4284892193 title "ZIF-67 derived Mo2N/Mo2C heterostructure as high-efficiency electrocatalyst for hydrogen evolution reaction" @default.
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- W4284892193 doi "https://doi.org/10.1016/j.jallcom.2022.166216" @default.
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