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- W4284959095 abstract "The present study describes the coating of modified graphite felt (GF) with graphene (GE) and polyaniline (PANI). GF was doped with nitrogen atoms by a series of modification and electrolytic deposition. Tests of different types of N content and cathodic catalytic oxidation performance confirmed that the graphite N introduction promoted the production of H2O2 in the 2e- process. Pyridine N catalyzed the H2O2 decomposition to produce •OH. The amount of H2O2 produced by GF, GF-GE, and [email protected] system was 11 mg L-1, 70 mg L-1, and 180 mg L-1, respectively. The doping of graphene increased H2O2 yield, and the electrolytic deposition of PANI converted H2O2 to •OH rapidly. It was proved that the N atom provided by graphene was graphite N, which was the active catalytic site for the production of H2O2. The perfluorooctanoic acid (PFOA) removal at 180 min was 24.1% and 49.8% in the GF and GF-GE systems, respectively. The [email protected] system achieved 100% PFOA removal within 160 min. It was demonstrated that the enrichment of PANI with pyridine N provided many active sites for improving the conversion of H2O2 to •OH and in-situ degrading organic pollutants, offering an alternative for wastewater treatment." @default.
- W4284959095 created "2022-07-10" @default.
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- W4284959095 date "2022-12-01" @default.
- W4284959095 modified "2023-10-16" @default.
- W4284959095 title "Electrochemical fabrication of polyaniline films deposited on graphene-loaded electrodes for •OH production and perfluorooctanoic acid degradation" @default.
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- W4284959095 doi "https://doi.org/10.1016/j.cej.2022.137914" @default.
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