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- W4284969346 abstract "Construction of effective charge separation and transfer channels is a critical issue in photocatalytic energy conversion. In this work, ultrasmall fine Pt nanoparticles and MoS2 nanosheets were deposited on the surface of g-C3N4 as cocatalysts. The presence of MoS2 can effectively induce the structural reconstruction of g-C3N4 and the redistribution of surface charges. The enriched electrons localized in the S and N atoms were conductive to the reduction of Pt4+ and the promotion of the metal–support interaction, thus boosting charge separation and transfer. As a result, the obtained Pt/MoS2/g-C3N4 composite provided a highly photocatalytic hydrogen activity, up to 1595.3 μmol h–1 with an AQE of 30.9% at 435 nm, 87.6 times higher than g-C3N4. This work may provide some insights into the rational design of high-efficient composite photocatalysts for solar energy conversion." @default.
- W4284969346 created "2022-07-10" @default.
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- W4284969346 date "2022-07-08" @default.
- W4284969346 modified "2023-10-17" @default.
- W4284969346 title "Interfacial Engineering of the Platinum/Molybdenum Disulfide/graphitic Carbon Nitride Composite for Enhanced Photocatalytic Hydrogen Production" @default.
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- W4284969346 doi "https://doi.org/10.1021/acsaem.2c01292" @default.
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