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- W4284976326 abstract "Based on thermoreversible sol–gel transitions of simple amino acid, fluorenylmethoxycarbonyl-modified phenylalanine (Fmoc-F), a hybrid double-network (DN) hydrogel, has been fabricated by combining a self-assembled Fmoc-F gel and a covalent polyacrylamide (PAAm) network. Up to 2 wt% Fmoc-F can be incorporated into DN hydrogels (90 wt% water) to form thinner and shorter nanofibers within the PAAm gel network than in pure Fmoc-F hydrogels; this indicates strong interaction between two gelators. Fmoc-F self-assembly also provides sacrificial bonding to effectively dissipate stretching energy, resulting in increased tensile modulus and yield strength of DN gels by 3437% and 737%, respectively, when compared with pure PAAm hydrogel. The relatively small increase of 133% and 177% in tensile strain and strength, respectively, of DN gels could be attributed to the time-independent discontinuous dissociation of the Fmoc-F self-assembly for energy dissipation. DN hydrogels also exhibit temperature-sensitive shape memory and self-recovery performance because of thermoreversible Fmoc-F self-assembly." @default.
- W4284976326 created "2022-07-10" @default.
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- W4284976326 date "2022-08-01" @default.
- W4284976326 modified "2023-10-02" @default.
- W4284976326 title "Fmoc-phenylalanine as a building block for hybrid double network hydrogels with enhanced mechanical properties, self-recovery, and shape memory capability" @default.
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- W4284976326 doi "https://doi.org/10.1016/j.polymer.2022.125145" @default.
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