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- W4285065777 endingPage "488" @default.
- W4285065777 startingPage "441" @default.
- W4285065777 abstract "Based on the theoretical gravimetric energy density of lithium-sulfur batteries (LiSBs) (2600 Wh kg− 1) and natural abundance and economic affordability of elemental sulfur, the all-solid-state lithium-sulfur batteries (SS-LiSBs) have a tremendous potential to assure powering from portable electronic devices to the heavy electric vehicles. Nevertheless, the use of traditional organic liquid electrolyte in lithium-sulfur batteries prevents them from being commercialized due to safety and several technical issues that are yet to be resolved. The major drawbacks are the formation of soluble lithium polysulfides (LiPS = Li2Sn), leading to poor cyclic performance, lower achievable capacity due to poor sulfur utilization, the low lithium-ion conductivity of the high sulfur-loaded electrode, the low electronic conductivity of sulfur as active material, and volume change during the charging/discharging process. High specific capacity (1166 mAh g− 1), competitive stability against volumetric variation corresponding to the charging/discharging process, higher melting point (938°C), and stable surface modification are significant advantages of Li2S as an alternative cathode material with the high potential for improving cyclic and rate performance of the Li-S batteries. Next, critical challenges and problems in practical applications, such as chemical and electrochemical stabilities, compatibility of solid-state electrolytes with the sulfur-based active materials, and lithium metal, are discussed. Finally, this chapter addresses improved safety, extended working temperature window, and high energy/power densities, which are several key advantages of SS-LiSBs." @default.
- W4285065777 created "2022-07-13" @default.
- W4285065777 creator A5038108109 @default.
- W4285065777 creator A5053718523 @default.
- W4285065777 creator A5073052948 @default.
- W4285065777 creator A5075023804 @default.
- W4285065777 creator A5078125230 @default.
- W4285065777 date "2022-01-01" @default.
- W4285065777 modified "2023-09-27" @default.
- W4285065777 title "A solid-state approach to a lithium-sulfur battery" @default.
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