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- W4285089773 abstract "We report on the synthesis, structure, and photophysical properties of a lead-free organic-inorganic hybrid halide, (Piperidinium)2MnBr4 (PipMBr). It crystallizes in a monoclinic P21/n structure, with isolated MnBr4 tetrahedra representing a zero-dimensional compound. It undergoes a reversible isostructural transition at 422/417 K in the heating/cooling cycle owing to the hydrogen-bonding rearrangement mediated by ring puckering of piperidinium cations. This compound exhibits green emission with a photoluminescence quantum yield of 51%. Interestingly, strong electron-longitudinal optical phonon coupling with γLO of 237 meV is evidenced from the broadening of the temperature-dependent emission linewidth and the Raman spectrum. Such strong electron-phonon coupling and a relatively low Debye temperature (137 K) suggest the self-trapped exciton emission in this compound." @default.
- W4285089773 created "2022-07-14" @default.
- W4285089773 creator A5021194769 @default.
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- W4285089773 date "2022-07-12" @default.
- W4285089773 modified "2023-09-29" @default.
- W4285089773 title "Zero-Dimensional (Piperidinium)<sub>2</sub>MnBr<sub>4</sub>: Ring Puckering-Induced Isostructural Transition and Strong Electron–Phonon Coupling-Mediated Self-Trapped Exciton Emission" @default.
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- W4285089773 doi "https://doi.org/10.1021/acs.inorgchem.2c01601" @default.
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