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- W4285289330 abstract "Hydrogen storage in metal organic frameworks (MOF) have generated a great deal of interest in recent years because of its exceptionally high specific surface area, pore volume and flexible surface chemistry. As per the guidelines of the US Department of Energy (DoE), for on-board hydrogen storage applications the adsorbent should exhibit a gravimetric capacity of 5.5 wt.% and volumetric capacity of 45 g L −1 , at an operating temperature of −40 to −60°C and a maximum pressure of 100 bar. In recent years, several MOFs were synthesized with gravimetric uptake much higher than that recommended by the US DoE. However, achieving the target volumetric capacity of 45 g L −1 is still a big challenge in most of these MOFs. Further, in these MOFs the desired targets are often achieved at cryogenic conditions such as 77 K. This put a serious constraint on the practical usage of these MOFs for hydrogen storage applications. Hence, in this chapter synthesis of new types of MOFs such as core shell MOFs, interpenetrated MOFs and composites based on MOF with nanoparticles are discussed. In addition, the recent strategies that are being adopted to improve the adsorption capacities of the existing MOFs is also explored. Further, techniques such as machine learning and other heuristic algorithms are currently being used to optimize the selection of these MOFs for hydrogen storage. The recent machine learning studies along with the future prospects of these MOFs toward commercial viability are also discussed in this chapter." @default.
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- W4285289330 date "2022-01-01" @default.
- W4285289330 modified "2023-10-01" @default.
- W4285289330 title "MOFs for hydrogen storage" @default.
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- W4285289330 doi "https://doi.org/10.1016/b978-0-323-91179-5.00019-x" @default.
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