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• W4285384414 endingPage "231835" @default.
• W4285384414 startingPage "231835" @default.
• W4285384414 abstract "Water management of membrane electrode assemblies (MEAs) has a significant impact on both the power performance and durability of anion exchange membrane fuel cells (AEMFCs). In this work, the hydrophobicity of catalyst layers (CLs) was systematically tuned using hydroxyl-functionalized and fluoroalkyl-functionalized carbon additives to improve water management. The inclusion of the fluorinated carbon in the anode CL effectively suppresses anode water flooding, whereas the hydroxyl-functionalized carbon additive in the cathode prevents cathode drying. The pairing of the hydrophobic anode CL and the hydrophilic cathode CL increases the maximum current density by 1.7 times compared with the carbon-additive-free MEA and ensures stable constant current operation for more than 1000 h due to the mitigation of water imbalance between the cathode and anode. This work highlights the importance of water management and provides simple and diversified means to tune the water distribution of an AEMFC. • Functionalized carbon additives affect the catalyst layer's hydrophobicity. • Hydrophobicity of catalyst layers affects the water condense behaviors. • The hydrophobic catalyst layer reduces the water flooding at the anode. • The hydrophilic catalyst layer prevents the water drying at the cathode. • Optimized water balance MEA exhibits superior performance and durability." @default.
• W4285384414 created "2022-07-14" @default.
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• W4285384414 date "2022-09-01" @default.
• W4285384414 modified "2023-10-16" @default.
• W4285384414 title "Tuning of water distribution in the membrane electrode assembly of anion exchange membrane fuel cells using functionalized carbon additives" @default.
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• W4285384414 doi "https://doi.org/10.1016/j.jpowsour.2022.231835" @default.
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