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• W4285392610 abstract "The reactions of FLPs with diazomethanes leads to the rapid loss of N2 . In contrast, in this work, we reported reactions of phosphine/borane FLPs with chlorodiazirines which led to the reduction of the N=N double bond, affording linked phosphinimide/amidoborate zwitterions of the general form R3 PNC(Ar)NR'BX(C6 F5 )2 . A detailed DFT mechanistic study showed that these reactions proceed via FLP addition to the N=N bond, followed by subsequent group transfer reactions to nitrogen and capture of the halide anion." @default.
• W4285392610 created "2022-07-14" @default.
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• W4285392610 date "2022-08-03" @default.
• W4285392610 modified "2023-10-17" @default.
• W4285392610 title "Reactions of Frustrated Lewis Pairs with Chloro‐Diazirines: Cleavage of N=N Double Bonds" @default.
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• W4285392610 doi "https://doi.org/10.1002/anie.202209241" @default.
• W4285392610 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35830598" @default.
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