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- W4285397855 abstract "Functional materials comprised of spontaneously self-assembled electron donor and acceptor entities capable of generating long-lived charge-separated states upon photo-illumination are in great demand as they are key in building the next generation of light energy harvesting devices. However, creating such well-defined architectures is challenging due to the intricate molecular design, multi-step synthesis, and issues associated in demonstrating long-lived electron transfer. Here, we have newly synthesized, by tether-directed functionalization, a [60]fullerene e -bisadduct carrying two Zn-porphyrins (Figure), and demonstrate supramolecular organization and photophysical events. Remarkably, the supramolecular assembly of the present bisporphyrin-C 60 forms donut-shape aggregates, primarily via π-π type charge transfer interactions. Upon photoexcitation, the supramolecular assembly generates long-lived charge-separated states of »1−40 μs lifetime due to electron/hole delocalization within the supramolecular structure Reference Caballero, M. Barrejón, J. Cerdá, J. Aragó, S. Seetharaman, P. de la Cruz, E. Ortí, F. D’Souza, F. Langa. J. Am. Chem. Soc. 2021, 143, 11199. Figure 1" @default.
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- W4285397855 date "2022-07-07" @default.
- W4285397855 modified "2023-09-30" @default.
- W4285397855 title "(Invited) Untethering the Tether Towards Spontaneously Self-Assembled Donuts" @default.
- W4285397855 doi "https://doi.org/10.1149/ma2022-0111827mtgabs" @default.
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